Yes, unsnarl is in the scrabble dictionary

...and is worth 11 points by itself.

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Unsnarl Definition

verb-transitive

To free of snarls; disentangle.
from The American Heritage Dictionary of the English Language, 4th Edition

verb

To disentangle a snarl in.
from Free Scrabble Dictionary

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Top Words by points

Points

unsnarl

7

2 letter words with UNSNARL

Points

an

2

al

2

nu

2

na

2

un

2

us

2

la

2

ar

2

as

2

3 letter words with UNSNARL

Points

sal

3

san

3

run

3

ras

3

ran

3

sau

3

sun

3

nus

3

nun

3

nan

3

als

3

ars

3

uns

3

urn

3

lun

3

las

3

lar

3

4 letter words with UNSNARL

Points

sunn

4

slur

4

sura

4

saul

4

ulan

4

nurl

4

ursa

4

ulna

4

urns

4

runs

4

nuns

4

nans

4

anus

4

larn

4

lars

4

luns

4

luna

4

5 letter words with UNSNARL

Points

nurls

5

ulnas

5

ulnar

5

ulans

5

annul

5

larns

5

sural

5

sunna

5

snarl

5

lunar

5

lunas

5

6 letter words with UNSNARL

Points

annuls

6

lunars

6

7 letter words with UNSNARL

Points

unsnarl

7

Found 57 words in 0.27712 seconds