Yes, unsure is in the scrabble dictionary

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Unsure Definition

adjective

Lacking confidence.
from The American Heritage Dictionary of the English Language, 4th Edition
Precarious; unstable; unreliable.
from The American Heritage Dictionary of the English Language, 4th Edition
Uncertain of the facts.
from The American Heritage Dictionary of the English Language, 4th Edition

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Top Words by points

Points

unsure

6

2 letter words with UNSURE

Points

er

2

un

2

us

2

en

2

re

2

nu

2

ne

2

es

2

3 letter words with UNSURE

Points

ers

3

sun

3

sue

3

ser

3

sen

3

uns

3

urn

3

ens

3

use

3

run

3

rue

3

res

3

ern

3

nus

3

4 letter words with UNSURE

Points

urns

4

urus

4

user

4

runs

4

sure

4

suer

4

ruse

4

rune

4

rues

4

erns

4

5 letter words with UNSURE

Points

runes

5

nurse

5

6 letter words with UNSURE

Points

unsure

6

Found 35 words in 0.22109 seconds